Never played any of the games, but I did watch every single Pokémon episode and movie (yeah, that’s over 1000 episodes rofl… 
). For OST I indeed have to agree with this one. Without this soundtrack some of the sad moments wouldn’t have been just as sad.
Some other classics that are among my favorites for OSTs:
Here a complete playlist for anyone going down the nostalgia train:
www.youtube.com/playlist?list=PL2E1A2C12F3A3B7D3
Off-topic, but for non-OST my top three Pokémon songs would be (albeit, maybe better suited for a separated thread):
- English first opening
- Japanese XYZ opening
- English (or maybe Dutch for nostalgia sake ) PokéRap endings
Greetz,
Quuador
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The one the sticks out for me most is Snowbelle city from X/Y. Nothing beats most the originals of coarse, but of the modern things I remember being greeted with this pleasant theme as you walk into the snowy town. So chill for me with the snow!
www.youtube.com/watch?v=UYObC_LRETk
Pokemon: Rise of Darkrai 2007 - Oracion OST. 
Pokemon: Jirachi-WishMaker - Make A Wish, 2003. ) im not old you’re old
www.youtube.com/watch?v=SGIfFdXthUs
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press play on all of these linked videos and listen to them at the same time
lavendertown. no question.
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bit late to the party but here and idk if they count since they’re remixes of a song.
I DON’T WANT TO SAY GOODBYE! Pokemon Mystery DUngeon.
Escape through the snow Pokemon Mystery Dungeon blue
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